More of Bobby's Greatest Hits is Bobby Vinton's second compilation of tracks from singles from 1964–1966. Nine of the ten tracks previously charted on the Billboard Hot 100, the lone exception being "Careless" which "bubbled under" (although it reached #82 on the competing Cashbox charts). The hits "Clinging Vine", "What Color (Is a Man)", "Dum-De-Da" and "Tears" (previously a hit for Ken Dodd) make their album debut on this compilation.